TY - JOUR
T1 - Size Ranges of Magnetic Domain States in Tetrataenite
AU - Mansbach, Elias N.
AU - Shah, Jay
AU - Williams, Wyn
AU - Maurel, Clara
AU - Bryson, James F. J.
AU - Weiss, Benjamin P.
N1 - Funding Information:
We acknowledge and thank funding from NASA FINESST Grant 80NSSC20K1366 and NASA contract NNM16AA09C, “Psyche: Journey to a Metal World.” We also acknowledge funding from the UK Natural Environment Research Council Grants (NERC) grants NE/S011978/1 and NE/S001018/1 to W.W. C.M. acknowledges the financial support of the European Marie Slokowska Curie Actions. We are grateful for the help of Dr. Santiago Benavides who provided assistance in setting up our modeling on the MIT Engaging Cluster. Additionally, we thank Les Nagy for productive conversations and suggestions for implementing MERRILL for this study. Lastly, we thank Rajesh Chopdekar and the Advance Light Source (ALS) at Lawrence Berkeley National Lab for setting up and maintaining the photon beam responsible for gathering our XPEEM data. This research used resources of the Advanced Light Source, a U.S. DOE Office of Science User Facility under contract no. DE‐AC02‐05CH11231.
Publisher Copyright:
© 2022 The Authors.
PY - 2022/10/17
Y1 - 2022/10/17
N2 - Paleomagnetic studies of meteorites provide unique constraints on the evolution of magnetic fields in the early solar system. These studies rely on the identification of magnetic minerals that can retain stable magnetizations over ≳4.5 billion years (Ga). The ferromagnetic mineral tetrataenite (γ''-Fe0.5Ni0.5) is found in iron, stony-iron and chondrite meteorite groups. Nanoscale intergrowths of tetrataenite have been shown to carry records of paleomagnetic fields, although the effect of magnetostatic interactions on their magnetic remanence acquisition remains to be fully understood. Tetrataenite can also occur as isolated, non-interacting, nanoscale grains in many meteorite groups, although the paleomagnetic potential of these grains is particularly poorly understood. Here, we aim to improve our understanding of tetrataenite magnetization to refine our knowledge of existing paleomagnetic analyses and broaden the spectrum of meteorite groups that can be used for paleomagnetic studies. We present the results of analytical calculations and micromagnetic modelling of isolated tetrataenite grains with various geometries. We find that tetrataenite forms a stable single domain state at grain lengths between 6 and ∼160 nm dependent on its elongation. It also possesses a magnetization resistant to viscous remagnetization over the lifetime of the solar system at 293 K. At larger grain sizes, tetrataenite’s lowest energy state is a lamellar two-domain state, stable at Ga-scale timescales. Unlike many other magnetic minerals, tetrataenite does not form a single-vortex domain state due to its large uniaxial anisotropy. Our results show that single domain and two-domain tetrataenite carries an extremely stable magnetization and therefore is a promising mineral for paleomagnetic studies.
AB - Paleomagnetic studies of meteorites provide unique constraints on the evolution of magnetic fields in the early solar system. These studies rely on the identification of magnetic minerals that can retain stable magnetizations over ≳4.5 billion years (Ga). The ferromagnetic mineral tetrataenite (γ''-Fe0.5Ni0.5) is found in iron, stony-iron and chondrite meteorite groups. Nanoscale intergrowths of tetrataenite have been shown to carry records of paleomagnetic fields, although the effect of magnetostatic interactions on their magnetic remanence acquisition remains to be fully understood. Tetrataenite can also occur as isolated, non-interacting, nanoscale grains in many meteorite groups, although the paleomagnetic potential of these grains is particularly poorly understood. Here, we aim to improve our understanding of tetrataenite magnetization to refine our knowledge of existing paleomagnetic analyses and broaden the spectrum of meteorite groups that can be used for paleomagnetic studies. We present the results of analytical calculations and micromagnetic modelling of isolated tetrataenite grains with various geometries. We find that tetrataenite forms a stable single domain state at grain lengths between 6 and ∼160 nm dependent on its elongation. It also possesses a magnetization resistant to viscous remagnetization over the lifetime of the solar system at 293 K. At larger grain sizes, tetrataenite’s lowest energy state is a lamellar two-domain state, stable at Ga-scale timescales. Unlike many other magnetic minerals, tetrataenite does not form a single-vortex domain state due to its large uniaxial anisotropy. Our results show that single domain and two-domain tetrataenite carries an extremely stable magnetization and therefore is a promising mineral for paleomagnetic studies.
U2 - 10.1029/2022GC010631
DO - 10.1029/2022GC010631
M3 - Article
VL - 23
JO - Geochemistry, Geophysics, Geosystems
JF - Geochemistry, Geophysics, Geosystems
SN - 1525-2027
IS - 11
M1 - e2022GC010631
ER -